A new class of tunable hypersonic phononic crystals based on polymer-tethered colloids
Identifieur interne : 000201 ( Main/Exploration ); précédent : 000200; suivant : 000202A new class of tunable hypersonic phononic crystals based on polymer-tethered colloids
Auteurs : E. Alonso-Redondo [Allemagne] ; M. Schmitt [États-Unis] ; Z. Urbach [Allemagne] ; C. M. Hui [États-Unis] ; R. Sainidou [France] ; P. Rembert [France] ; K. Matyjaszewski [États-Unis] ; M. R. Bockstaller [États-Unis] ; G. Fytas [Allemagne, Grèce]Source :
- Nature Communications [ 2041-1723 ] ; 2015.
Abstract
The design and engineering of hybrid materials exhibiting tailored phononic band gaps are fundamentally relevant to innovative material technologies in areas ranging from acoustics to thermo-optic devices. Phononic hybridization gaps, originating from the anti-crossing between local resonant and propagating modes, have attracted particular interest because of their relative robustness to structural disorder and the associated benefit to ‘manufacturability'. Although hybridization gap materials are well known, their economic fabrication and efficient control of the gap frequency have remained elusive because of the limited property variability and expensive fabrication methodologies. Here we report a new strategy to realize hybridization gap materials by harnessing the ‘anisotropic elasticity' across the particle–polymer interface in densely polymer-tethered colloidal particles. Theoretical and Brillouin scattering analysis confirm both the robustness to disorder and the tunability of the resulting hybridization gap and provide guidelines for the economic synthesis of new materials with deliberately controlled gap position and width frequencies.
Url:
DOI: 10.1038/ncomms9309
PubMed: 26390851
PubMed Central: 4595630
Affiliations:
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Sainidou</name><affiliation wicri:level="1"><nlm:aff id="a4"><institution>Laboratoire Ondes et Milieux Complexes, UMR CNRS 6294, University of Le Havre</institution>, 75 Rue Bellot, 76600 Le Havre,<country>France</country></nlm:aff><country xml:lang="fr">France</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Rembert, P" sort="Rembert, P" uniqKey="Rembert P" first="P." last="Rembert">P. Rembert</name><affiliation wicri:level="1"><nlm:aff id="a4"><institution>Laboratoire Ondes et Milieux Complexes, UMR CNRS 6294, University of Le Havre</institution>, 75 Rue Bellot, 76600 Le Havre,<country>France</country></nlm:aff><country xml:lang="fr">France</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Matyjaszewski, K" sort="Matyjaszewski, K" uniqKey="Matyjaszewski K" first="K." last="Matyjaszewski">K. Matyjaszewski</name><affiliation wicri:level="1"><nlm:aff id="a3"><institution>Department of Chemistry, Carnegie Mellon University</institution>, 4400 Fifth Avenue, Pittsburgh, Pennsylvania 15213, USA</nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea>, 4400 Fifth Avenue, Pittsburgh, Pennsylvania 15213</wicri:regionArea><wicri:noRegion>Pennsylvania 15213</wicri:noRegion></affiliation></author><author><name sortKey="Bockstaller, M R" sort="Bockstaller, M R" uniqKey="Bockstaller M" first="M. R." last="Bockstaller">M. R. Bockstaller</name><affiliation wicri:level="1"><nlm:aff id="a2"><institution>Department of Materials Science and Engineering, Carnegie Mellon University</institution>, 5000 Forbes Avenue, Pittsburgh, Pennsylvania 15213, USA</nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea>, 5000 Forbes Avenue, Pittsburgh, Pennsylvania 15213</wicri:regionArea><wicri:noRegion>Pennsylvania 15213</wicri:noRegion></affiliation></author><author><name sortKey="Fytas, G" sort="Fytas, G" uniqKey="Fytas G" first="G." last="Fytas">G. Fytas</name><affiliation wicri:level="1"><nlm:aff id="a1"><institution>Max Planck Institute for Polymer Research</institution>, Ackermannweg 10, 55128 Mainz,<country>Germany</country></nlm:aff><country xml:lang="fr">Allemagne</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation><affiliation wicri:level="1"><nlm:aff id="a5"><institution>Department of Materials Science, FORTH-IESL,</institution> PO Box 1527, 71110 Heraklion,<country>Greece</country></nlm:aff><country xml:lang="fr">Grèce</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author></analytic><series><title level="j">Nature Communications</title><idno type="eISSN">2041-1723</idno><imprint><date when="2015">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>The design and engineering of hybrid materials exhibiting tailored phononic band gaps are fundamentally relevant to innovative material technologies in areas ranging from acoustics to thermo-optic devices. Phononic hybridization gaps, originating from the anti-crossing between local resonant and propagating modes, have attracted particular interest because of their relative robustness to structural disorder and the associated benefit to ‘manufacturability'. Although hybridization gap materials are well known, their economic fabrication and efficient control of the gap frequency have remained elusive because of the limited property variability and expensive fabrication methodologies. Here we report a new strategy to realize hybridization gap materials by harnessing the ‘anisotropic elasticity' across the particle–polymer interface in densely polymer-tethered colloidal particles. Theoretical and Brillouin scattering analysis confirm both the robustness to disorder and the tunability of the resulting hybridization gap and provide guidelines for the economic synthesis of new materials with deliberately controlled gap position and width frequencies.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Maldovan, M" uniqKey="Maldovan M">M. Maldovan</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Han, T" uniqKey="Han T">T. Han</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Xu, H" uniqKey="Xu H">H. Xu</name></author><author><name sortKey="Shi, X" uniqKey="Shi X">X. Shi</name></author><author><name sortKey="Gao, F" uniqKey="Gao F">F. Gao</name></author><author><name sortKey="Sun, H" uniqKey="Sun H">H. Sun</name></author><author><name sortKey="Zhang, B" uniqKey="Zhang B">B. 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